Catalytic Materials: Relationship Between Structure and Reactivity

Editor(s): Thaddeus E. Whyte, Jr., Ralph A. Dalla Betta, Eric G. Derouane, and R. T. K. Baker. Volume 248. Publication Date (Print): April 5, 1984. IS...
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Catalytic Materials: Relationship Between Structure and Reactivity

ACS

SYMPOSIUM

SERIES

248

Catalytic Materials: Relationship Between Structure and Reactivity Thaddeus E. Whyte, Jr., EDITOR Catalytica Associates, Inc.

Ralph A. Dalla Betta, EDITOR Catalytica Associates, Inc.

Eric G. Derouane, EDITOR Mobil Technical Center

R. T. K. Baker, EDITOR Exxon Research & Engineering Co. Based on the 1983 State-of-the-Art Symposium sponsored by the Division of Industrial and Engineering Chemistry, San Francisco, California, June 13-16, 1983

American Chemical Society, Washington, D.C. 1984

Library of Congress Cataloging in Publication Data Catalytic materials. (ACS symposium series, ISSN 0097-6156; 248) "Based on the 1983 state-of-the-art symposium sponsored by the Division of Industrial and Engineering Chemistry, San Francisco, California, June 13-16, 1983." Includes bibliographies and indexes. 1. Catalysts—Congresses. I. Whyte, Thaddeus Ε., 1937. II. American Chemical Society. Division of Industrial and Engineering. III. Series. QD505.C387 1984 ISBN 0-8412-0831-X

541.3'95

84-2776

Copyright © 1984 American Chemical Society All Rights Reserved. The appearance of the code at the bottom of the first page of each chapter in this volume indicates the copyright owner's consent that reprographic copies of the chapter may be made for personal or internal use or for the personal or internal use of specific clients. This consent is given on the condition, however, that the copier pay the stated per copy fee through the Copyright Clearance Center, Inc., 21 Congress Street, Salem, M A 01970, for copying beyond that permitted by Sections 107 or 108 of the U.S. Copyright Law. This consent does not extend to copying or transmission by any means—graphic or electronic—for any other purpose, such as for general distribution, for advertising or promotional purposes, for creating a new collective work, for resale, or for information storage and retrieval systems. The copying fee for each chapter is indicated in the code at the bottom of the first page of the chapter. The citation of trade names and/or names of manufacturers in this publication is not to be construed as an endorsement or as approval by ACS of the commercial products or services referenced herein; nor should the mere reference herein to any drawing, specification, chemical process, or other data be regarded as a license or as a conveyance of any right or permission, to the holder, reader, or any other person or corporation, to manufacture, reproduce, use, or sell any patented invention or copyrighted work that may in any way be related thereto. Registered names, trademarks, etc., used in this publication, even without specific indication thereof, are not to be considered unprotected by law. P R I N T E D IN THE U N I T E D STATES O F A M E R I C A

ACS Symposium Series M. Joan Comstock, Series Editor Advisory Board Robert Baker U.S. Geological Survey

Geoffrey D. Parfitt Carnegie-Mellon University

Martin L . Gorbaty Exxon Research and Engineering Co.

Theodore Provder Glidden Coatings and Resins

Herbert D. Kaesz University of California— Los Angeles

James C. Randall Phillips Petroleum Company

Rudolph J. Marcus Office of Naval Research

Charles N. Satterfield Massachusetts Institute of Technology

Marvin Margoshes Technicon Instruments Corporation

Dennis Schuetzle Ford Motor Company Research Laboratory

Donald E . Moreland USDA, Agricultural Research Service W. H . Norton J. T. Baker Chemical Company Robert Ory USDA, Southern Regional Research Center

Davis L . Temple, Jr. Mead Johnson Charles S. Tuesday General Motors Research Laboratory C. Grant Willson IBM Research Department

FOREWORD The

A C S SYMPOSIUM SERIES w a s f o u n d e d i n 1974 to p r o v i d e

a m e d i u m for p u b l i s h i n g s y m p o s i a q u i c k l y i n b o o k f o r m . T h e f o r m a t of the Series p a r a l l e l s t h a t of t h e c o n t i n u i n g ADVANCES IN CHEMISTRY SERIES e x c e p t t h a t i n o r d e r to save t i m e p a p e r s are n o t typeset b u t are r e p r o d u c e d as t h e y are m i t t e d b y the authors i n c a m e r a - r e a d y f o r m . P a p e r s are

the sub­ re­

v i e w e d u n d e r the s u p e r v i s i o n of the E d i t o r s w i t h t h e assistance of the Series A d v i s o r y B o a r d a n d are s e l e c t e d to m a i n t a i n t h e i n t e g r i t y of the s y m p o s i a ; h o w e v e r , v e r b a t i m r e p r o d u c t i o n s of p r e v i o u s l y p u b l i s h e d p a p e r s are n o t a c c e p t e d . B o t h r e v i e w s a n d reports

of r e s e a r c h are a c c e p t a b l e

e m b r a c e b o t h types of p r e s e n t a t i o n .

since s y m p o s i a m a y