Designed Polar Cosolvent-Modified Supercritical CO2 Removing

Lea , M.; Xiao , Q.; Sadhukhan , A.; Cottle , S.; Wang , Z. Y.; Yang , C. S. Inhibition effects of green tea extracts and (–)epigallocatechin gallat...
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9014

J. Agric. Food Chem. 2007, 55, 9014–9020

Designed Polar Cosolvent-Modified Supercritical CO2 Removing Caffeine from and Retaining Catechins in Green Tea Powder Using Response Surface Methodology KUO-JONG HUANG,† JIA-JIUAN WU,§ YUNG-HO CHIU,# CHENG-YUNG LAI,‡ CHIEH-MING J. CHANG*,†

AND

Department of Chemical Engineering, National Chung Hsing University, 250 Kuo-Kuang Road, Taichung, Taiwan 402, Republic of China; Department of Nutrition, China Medical University, 91 Hsueh-Shih Road, Taichung, Taiwan 404, Republic of China; Department of Research and Development, Taiwan Supercritical Technology Company, Ltd., 346 Yuan-Tsao Road, Changhua, Taiwan 502, Republic of China; and Chihlee Institute of Technology, Banciao, Taiwan 220, Republic of China

This study examines cosolvent-modified supercritical carbon dioxide (SC-CO2) to remove caffeine from and to retain catechins in green tea powder. The response surface method was adopted to determine the optimal operation conditions in terms of the extraction efficiencies and concentration factors of caffeine and catechins during the extractions. When SC-CO2 was used at 333 K and 300 bar, 91.5% of the caffeine was removed and 80.8% of catechins were retained in the tea: 3600 g of carbon dioxide was used in the extraction of 4 g of tea soaked with 1 g of water. Under the same extraction conditions, 10 g of water was added to