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Consistent and Effective Nonlinearity Index and its Application on Model Predictive Controller Performance Deterioration Fahim Uddin, Lemma Dendena Tufa, and Abdulhalim Shah Maulud Ind. Eng. Chem. Res., Just Accepted Manuscript • DOI: 10.1021/acs.iecr.8b01984 • Publication Date (Web): 06 Oct 2018 Downloaded from http://pubs.acs.org on October 8, 2018
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Industrial & Engineering Chemistry Research
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Consistent and Effective Nonlinearity Index and its
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Application on Model Predictive Controller
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Performance Deterioration Fahim Uddin1, Lemma Dendena Tufa1,* Abdulhalim Shah Maulud1
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Chemical Engineering Department, Universiti Teknologi PETRONAS, Seri Iskandar - 32610,
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Perak Darul Ridzuan, Malaysia
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Keywords: Nonlinearity, Nonlinearity Index, Model Predictive Control, Aspen Plus.
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Abstract
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Many control-relevant systems present the challenges of nonlinearity, directionality and ill-
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conditioning for the control systems, and exhibit poor controller performance. This study
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proposes a Nonlinearity Index to quantify the extent of nonlinearity of such systems. A dynamic
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nonlinear model of a pilot-scale distillation column operating near the azeotropic region was
*
Corresponding author
Lemma Dendena Tufa, E-mail:
[email protected], Contact # 060-12-2696 816
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simulated using Aspen Plus Dynamics. A comparison of the results is made with the
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Nonlinearity Measure proposed by Du et al. Results show that a significant increase is exhibited
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in the proposed nonlinearity index values of the system as the system moves towards the
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azeotropic region. Prediction errors of the linear models are also shown to be correlated to the
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proposed index. Therefore, the proposed Nonlinearity Index is consistent with the existing
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indicators of nonlinearity, and thus its measurements of system nonlinearity are reliable.
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Controller performance for the system at higher values of the proposed index further presents its
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efficacy.
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1. Introduction
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Nonlinearity of the system has always been a concern for system identification, analysis and
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control 1-2. Mildly nonlinear systems can be approximated as linear systems and thus can
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effectively be controlled using quasi-linear filtering methods. Whereas, a highly nonlinear
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system can only be represented effectively by a nonlinear model and thus requires nonlinear
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filtering. Linear controllers of such plants will always perform poorly and high model-plant
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mismatches (MPMs) will be detected by the MPM algorithms. Moreover, such algorithms are
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not sufficient for the performance improvement of highly nonlinear systems 3-5. As nonlinear
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filtering results in high computation and complexity, it is desirable to avoid nonlinear filtering as
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much as feasible. This can be achieved by determining the degree of system nonlinearity, which
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can categorise whether the system has sufficient nonlinearity to require a nonlinear control
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structure. However, the quantification of the extent of nonlinearity has not been studied
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extensively, and there is a lot of scope for determining parameters which can evaluate the
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nonlinearity of the system effectively.
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Nonlinearity is not only displayed by the real systems but also can be found in the first-
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principle models of these systems. Such systems, although conveniently simulated by
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commercially available simulators such as Aspen HYSYS®, Aspen Plus® and MATLAB®, are
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found to be challenging for linear control 6-8. Since these simulations are able to demonstrate the
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dynamic behaviour of the plant, they are widely used in chemical engineering applications for
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conceptualisation, analysis, identification and control 9-11.
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A general classification of the existing nonlinearity indices (NLIs) is as follows:
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1.
Distance from the closest linear model
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2.
Function of Nonlinear curvature around any operating point.
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3.
Nonlinearity tests (only determine if a system is nonlinear, not its degree)
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The idea to measure nonlinearity based on its distance from a linear approximation was
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introduced by Beale in 1960, who used regression analysis for the purpose 12. Later on, an NLI
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for systems involving inverse scattering was proposed as the absolute magnitude of the product
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of diagonal operators and internal radiation terms of the Neumann series expansion 13.
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NLIs based on the distance between a nonlinear system and its best linear approximation were
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presented by 14-18. A normalised version of 14 was proposed by 19, however, its computation
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required a numerical solution, and thus the authors of 20 proposed to calculate a similar NLI
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using functional expansions. Controllability and observability gramians of the linearised system
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were also proposed to determine nonlinearity of the system 21.
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Use of two linear systems for nonlinearity measurement was proposed 18. In this method, NLI
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is the larger of the distances from N to its greatest-lower and the smallest-upper linear boundary 3 ACS Paragon Plus Environment
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function. However, the extension of this method to multiple-input-multiple-output (MIMO)
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systems is challenging, and determination of the linear boundary functions can prove to be
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difficult 22. Liu et al. 23 proposes an NLI as the minimum distance from the set of all linear
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models. This NLI is able to deal with additive and non-additive noise.
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Gap metric was introduced, which is the distance between the linear approximation of the
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nonlinear system and another linear system 24-26. Applications of this metric for nonlinearity
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estimation and multimodel control have been studied 27-28 via weight-based control 29, the H∞
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loop-shaping technique 30, stability margin 31-32 and integration with the neighbourhood
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estimation algorithm33. However, linearization may lose an important part of the nonlinearity
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which is detrimental for the appropriate nonlinearity measurement.
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Instead of the distance of the system from its linear approximation, some researchers prefer to
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use the decline of control performance as a direct measure of the nonlinearity. This performance
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decline can also be considered as the distance from the linear model in terms of control
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performance. A ‘Performance Sensitivity Measure’ was introduced which basically is an index to
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measure the control-relevant nonlinearity by quantifying the performance loss of linear quadratic
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gaussian (LQG) controller 34. This work was further extended in 35. This measure uses the first
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and second order sensitivity coefficients, which are obtained using the original nonlinear first-
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principle models. However, this methodology has not been extended to the nonlinear systems
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whose first-principle models are not present or difficult to obtain. Two local nonlinearity indices
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were proposed which measure the departure of LQG controller performance and stability from
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optimality 36. These indices were able to be integrated with the control design. Another index
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used the variance in the disturbance rejection performance of a linear controller to measure the
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nonlinearity in an operating range 37. This index was shown to be better than the gap metric for 4 ACS Paragon Plus Environment
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determination of nonlinearity. The lower bound ratio of the minimum variance was also
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proposed as a measure of control-relevant nonlinearity 38. The method is data-driven and is
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applicable to Wiener, Hammerstein and Wiener-Hammerstein structures.
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The advantage of NLIs in this class is that they usually do not require the derivative of the function. However, they have several drawbacks: 23
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1.
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They usually present the worst-case scenario, which may be very different from the normal operation.
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2.
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They are not suited for estimation as they do not account for the randomness of the estimated quantity.
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3.
They usually require high computation and are thus inappropriate for MIMO systems.
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Another way to calculate NLI is to utilise the curvature from differential geometry. Refs. 39-40
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defined an NLI based on curvature, which uses its first and second derivatives. Both of these NLI
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curvatures were calculated 41 and applied to various real-world problems 42-45, and performance
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evaluation based on NLI curvatures was also carried out 46. Another index measured the steady-
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state nonlinearity using partial differentiation 47. The tangential and normal components were
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used to determine the nonlinearity of the process.
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The advantages of curvature-based NLIs are 23:
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1. They are relatively easier to compute in case of easy/defined derivatives.
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2.
They are easy to visualise geometrically.
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3.
Intrinsic curvature is independent of parametrisation.
However, they also incur various disadvantages, such as 23:
99 100
1.
The derivatives must be determined analytically.
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2.
They provide a pessimistic measure of nonlinearity since they usually calculate the
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maximum nonlinearity present in the system at a particular frequency which might
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not be helpful or relevant to a specific control application.
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3.
They ignore high order terms, which also contribute to system nonlinearity.
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Mixed-filtering based NLI was proposed 48, in which a linear and a nonlinear filter were
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applied in parallel and summed. A minimisation function determines the weights of the sum,
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where the weight of nonlinear filter is referred to as NLI. However, its dependence on the filter
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selection and representation of the performance rather than nonlinearity are not justified.
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One way to determine the nonlinearity is to apply any of the several nonlinearity tests
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proposed in the literature 49-54 to the time series or clinical data. These tests determine whether
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the system is linear or not without providing insights to the degree of nonlinearity. However,
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having an estimate of the extent of nonlinearity is more informative than just knowing whether
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the system is nonlinear. The current study adopts the idea of 50 and transforms it into a
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measurable index of nonlinearity for MIMO systems which can assess whether the linear process
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control of a system will fail to deliver acceptable performance. This index is then compared with
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an existing nonlinearity index in the literature and their relationship with the parameters
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indicating system nonlinearity are observed. The NLI-proposed degree of nonlinearity of the
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operating ranges is also tested by observing the system control behaviours of these ranges.
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The rest of the paper is arranged as follows: Section 2 explains the mathematical derivation
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and input requirements of the proposed nonlinearity index. Section 3 discusses the development
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of the case study, its control structure and data generation for the measurement of nonlinearity.
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An existing nonlinearity measure (NM) from the literature is also briefly introduced. Section 4
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presents the results obtained by the application of proposed NLI. The values of the proposed NLI 6 ACS Paragon Plus Environment
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and NM are compared for various operating ranges, input magnitudes and linear model
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prediction errors. Control performance of the system at different NLI values are also shown.
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Finally, Section 5 presents the conclusion of this study.
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2. Current Work
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2.1. Proposed Nonlinearity Index
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A test statistic was introduced by Billings and Voon50 in order to determine the structure of the
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system. In this statistic, the higher order correlation functions were used and compared against
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the maximum allowable value for 95% confidence limits. The test requires that the input u(t) and
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noise e(t) are independent, with their means and odd-order moments being zero. These properties
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can be ensured by using sine wave, gaussian signal, ternary pseudorandom sequence or
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independent uniformly distributed process as the input signal. The correlation function ϕ at delay
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or lags τ between N number of measured values of output with sample mean as 𝑦 is defined as:
yy
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yy
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2
2
( )
( )
E[( y( k ) y )( y( k ) y ) 2 ] 1 N
N
[( y
( k )
k
y )( y( k ) y ) 2 ]
(1) (2)
If the system is perfectly linear, the odd order moments of the output signal obtained will also
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be zero. Consequently, it was proposed using 95% confidence limits that any dynamic system
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can be appropriately represented by a linear model if:
yy
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2
( )
yy (0) y
2 2
y (0)
1.96 N
(3)
According to Billings and Voon 50, the left-hand side of the equation needs to be evaluated and
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checked whether it exceeds the threshold set on the right-hand side of the equation. However,
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this does not provide any information on the extent of nonlinearity.
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In order to measure the extent of nonlinearity, this equation can be rearranged for this work as: 8 ACS Paragon Plus Environment
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0.5102 N
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yy
2
( )
yy (0) y
1 y (0)
Defining the proposed Nonlinearity Index as:
NLI 0.5102 N
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yy
2
( )
yy (0) y
(5) 2 2
y (0)
where an NLI value of zero represents absolute linearity and one represents sufficient
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nonlinearity to use nonlinear model for identification. Since it is a ratio of odd and even order
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moments, the units cancel each other and the resulting NLI carries no units.
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(4)
2 2
In order to define overall nonlinearity of a MIMO system having j number of outputs, a general expression is defined as: j
1 j
NLI (1 NLI yi ) 1
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(6)
i 1
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2.2. Plant Excitation for NLI measurements
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The nonlinearity test defined in section 2.1 requires that the input signals must have zero odd-
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order moments 50. Therefore, sine wave signals can be used for the excitation of the system.
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Consequently, the amplitudes of inputs sine waves are varied systematically using appropriate
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step size and introduced to the selected operating regimes. It is better to keep the inputs out of
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phase and to have different frequencies in order to explore the interaction of the system.
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3. Case Study: Nonlinearity Measurement near Azeotropic Region
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In order to demonstrate the effectiveness of the proposed nonlinearity index (NLI), distillation
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column control near azeotropic region is selected as the case study. It has been observed in our
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previous work 55 that as the system moves towards the azeotropic region, the following
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observations are made:
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1.
As the operating range moves near high purity/azeotropic point, the nonlinearity of
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the system increases. Hence it is difficult to present the system behaviour effectively
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using any linear model.
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2.
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system.
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3.
175 4.
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As the nonlinearity increases, the prediction accuracy of any linear model identified for the system decreases.
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The wider the operating range gets, the more the nonlinearity is incurred by the
Since controller performance is adversely affected by nonlinearity, any increase in the nonlinearity results in a decrease in control performance.
The magnitude of the proposed NLI is defined to be proportional to the actual nonlinearity of the system, therefore it should be able to achieve the following results.
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1.
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Proposed nonlinearity index should represent an increase in nonlinearity of the system as the operating range moves towards azeotropic point.
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2.
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Proposed nonlinearity index should indicate an increase in nonlinearity as the operating range of the system gets wider.
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3.
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For higher values of the proposed nonlinearity index, the prediction error of the linear model identified for the system should increase.
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4.
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Increase in the value of the proposed nonlinearity index should result in a decrease in control performance.
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In order to analyse the relevance of NLI as the system moves towards the azeotropic region,
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three different operating regimes with different steady states were selected, differing only in the
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steady-state compositions. Consequently, three Aspen Plus® simulations were developed. These
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simulations were then converted to dynamic mode, and Model Predictive Control (MPC) was
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designed for the top and bottom compositions.
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3.1. Aspen Plus® Dynamic Simulation
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This study was conducted by using Aspen Plus® dynamic simulation of the pilot distillation
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column present at Universiti Teknologi PETRONAS as presented in Figure 1. The column has
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15 stages, 0.35 m apart, with the feed entering at the ninth stage. The ethanol-water separation
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using this column was selected for this study. The feed of binary mixture, composed of 25 mol%
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ethanol with a flow rate of 0.6 m3/hr, enters the column T-300 through feed valve F3-V at 77oC.
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The ethanol-enriched stream is collected as distillate after being condensed. The pressure in the
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condenser was maintained at 1.25 bar to reflect the near-atmospheric distillation systems. A
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detailed account of the development of steady-state simulation for this pilot plant has been
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reported in the literature 11, 56. The column results for the selected operating regimes have been
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summarized in Table 1. The major difference among the operating regimes is the ethanol
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composition among the distillate streams of the operating regimes as shown in Table 2. 11 ACS Paragon Plus Environment
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Figure 1: Process Schematic for the Aspen Plus® Dynamic Simulation of Pilot-Plant Distillation
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Column
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Table 1: Steady-state stream conditions of the simulations Stream conditions
Feed
Distillate
Bottoms
Temperature (C)
77
83.56
91.20
Pressure (kPa)
130.95
124.75
135.78
Flowrate (m3/hr)
0.6
0.13044
0.4806
209 210
Table 2: Ethanol compositions Operating Regimes
SS-82
SS-83
SS-84
Feed (Steady state)
25
25
25
Distillate (Steady state)
82.01
83.02
83.99
Bottoms (Steady state)
17.42
17.35
17.29
Operating Ranges
[80.75 83.25]
[81.75 84.25]
[82.75 85.25]
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The pressure-driven dynamic simulation had a pressure controller as a default in the
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simulations. This proportional-integral (PI) controller maintained the pressure of the condenser
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by manipulating condenser duty. A PI feed flowrate controller and two proportional (P) level
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controllers for the condenser and reboiler level were installed in each simulation. Details
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regarding the general setup procedure for dynamic simulations can be found in the literature 8, 57,
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whereas the configurations of P and PI controllers can be found in 58.
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3.2. Data Generation for NLI Calculation
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In order to generate data for the calculation of proposed NLI, the sine inputs are entered in the
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system for six hours, generating a total number of 600 data samples for analysis, using 0.01 hr as
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sample time. Sine inputs with amplitudes varying from 5% to 20% were used to observe the NLI
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for different widths of operating ranges. Sine inputs with amplitudes of 5% as well as 20% are
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plotted in Figure 2 for illustration.
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Figure 2: Input sequences to the simulation for NLI calculation
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3.3. NM Calculation The nonlinearity measure proposed by Du et al. 59 is compared with the proposed NLI. The
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comparison will be made based on the ability to show a consistent increase in system
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nonlinearity as the system moves towards the azeotropic region or widens the existing operating
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range. According to Du et al. 59, the nonlinearity measure can be calculated by the following
231
equation:
NM
232
max ( P*)
(7)
bP*, K
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Where δmax (P*) is the Maximum gap i.e. Gap metric of the system and bP*,K is the gap metric
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stability margin of the system P* and linearized stable controller K, which is given by the
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following expression: bP , K
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I 1 K I PK I
1
P
I 1 P I KP I
1
K
(8)
As the gap metric stability margin is a function of the system as well as the controller,
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appropriate control configuration is required for its calculation. Therefore, proportional-integral-
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derivative (PID) controller configurations were identified using MATLAB® command ‘pidtune’
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for PID controller design and used for the calculation. This command selects PID tuning to
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ensure appropriate open-loop phase margin as well as cross-over frequency for a given system.
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3.4. System Identification and Control
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The plant is excited using Pseudo Random Binary Signal (PRBS) for the development of linear models of the operating regimes for model predictive control, as shown in Figure 3. In order to 15 ACS Paragon Plus Environment
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avoid ill-conditioned modelling of the system, the outputs i.e. top composition yD and bottom
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composition yB, inputs i.e. reflux flowrate R and reboiler duty QB and disturbance i.e. feed
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flowrate F were scaled as follows:
a'
248 249
a a SS aR
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(9)
Where aSS is the steady-state value of the parameter and aR is its span.
250 251 252 253 254
255
256
Figure 3: Input sequences and output responses for System Identification The 2x3 first order plus time delay (FOPTD) models were identified as shown in the following equations. Note that the delays less than the sampling time Ts=0.01 hr were neglected. For the operating regime SS-82, 4.146 y 'D 0.085s 1 y ' 1.179 B 0.198s 1
4.327 1.519 0.084 s 1 R ' 0.129 s 1 F' 1.668 Q 'B 0.9723 0.198s 1 0.195s 1
For the operating regime SS-83, 16 ACS Paragon Plus Environment
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2.03 y 'D 0.067 s 1 y ' 0.921 B 0.197 s 1
257
258
(11)
0.962 0.3147 R ' 0.586 s 1 0.084 s 1 F' 0.907 Q 'B 0.9199 0.207 s 1 0.196 s 1
(12)
For the operating regime SS-84, 3.891 y ' D 0.276 s 1 y ' 3.270 B 0.206 s 1
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260
2.578 0.1236e 0.08 s 0.069 s 1 R ' 0.03s 1 F' 1.419 Q 'B 0.9653 0.189 s 1 0.197 s 1
Where y’D and y’B are the scaled outputs i.e. top and bottom compositions, R’ and Q’B are the
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scaled inputs i.e. reflux flowrate and reboiler duty and F’ is the scaled disturbance i.e. feed
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flowrate.
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Table 3 shows that the models for the selected regimes fitted more than 95% to estimation data
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of output yD and 80% to estimation data of output yB, using prediction focus. It can be observed
265
that the identified models for the selected regimes fit the identification data well. The Final
266
Prediction Error (FPE) and Mean Square Error (MSE) were found to be of the order of 10-11 and
267
10-6 respectively for the selected regimes. The Relative Gains (RG) for these models suggest that
268
the top composition (yD) is more influenced by reflux (R) than by the reboiler duty (QB) in all the
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cases, which is in accordance with the intuition.
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Table 3: Comparison of the identified models Model Accuracy
SS-82
SS-83
SS-84
Fit% (prediction focus)
[95.74;97.4]
[96.5;97.6]
[95.8;97.2]
FPE × 1011
1.918
2.092
4.790
MSE × 106
12.76
8.646
7.435
Relative Gain
3.81
5.69
0.53
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Using these models, suitable MPCs are designed for composition control as shown in Table 4.
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Tuning advisor is used from MATLAB MPC toolbox for the controller tuning. Therefore, the
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system is ready for the evaluation of controller performance. For setpoint tracking performance,
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the system will incur a step change in the setpoint, the magnitude of which will depend on the
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operating range. For disturbance rejection, a step change in disturbance will be introduced to the
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system.
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Table 4: Tuning parameters selected for MPC using Tuning advisor Tuning parameters
SS-82
SS-83
SS-84
Sampling Time
0.01 hr
0.01 hr
0.01 hr
Prediction Horizon
30
30
30
Control Horizon
10
10
10
Output Weights
[3.75 1.85]
[2.15 1.88]
[2.15 1.88]
Input Weights
[0 0]
[0 0]
[0 0]
Input Rate Weights
[1.5 0.5]
[1.5 0.5]
[1.5 0.5]
279 280
4. Results and Discussions
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4.1. Perturbation Responses for Determining NLI
282
Figure 4 presents the Aspen Plus simulation responses for the operating regimes SS-82, SS-83
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and SS-84 for the inputs shown in Figure 2. It is observed that the systems show relatively
284
deterministic linear behaviour when the input amplitudes are low. For higher input values, the
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systems show increased nonlinear response. The responses of the system observed in this section
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are utilised for the calculation of the proposed NLI for the system.
287 288
Figure 4: Output responses of the Aspen Plus® Dynamic Simulation
289
4.2. Variation w.r.t. Input Magnitude and Distance from the Azeotropic Region
290
291
The system is ready to be evaluated by the proposed NLI for its extent of nonlinearity by using
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the data from Section 4.1. A comparison with a recently proposed nonlinearity measure (NM) by
293
Du et al. (2017) 59 is also made to further demonstrate the efficacy of NLI.
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The values of the NLI proposed in this study are shown in Table 5. Effects of input magnitudes
295
and distance from the azeotropic point are observed. Since the nonlinearity index has been
296
defined to use the open-loop sinusoidal inputs and its responses, it is relevant to compare the
297
values of nonlinearity index for different operating regimes against same input perturbations in
298
open loop. As required, the NLI values are found to increase with an increase in input
299
magnitude, as well as with the decrement of distance from the azeotropic region.
300
It can be realised from Figure 5 that the values of the nonlinearity index for SS-82 are less than
301
one for all input magnitudes, which means that this operating range can be considered a linear
302
system. A maximum value of 0.90 was observed, which is still below the statistical limit of 1. A
303
linear model is sufficient for acceptable control performance using the model predictive control in
304
such cases. On the other hand, the NLI value of the regime SS-84 for 20% input magnitude is
305
greater than one, which means that a nonlinear model is required for acceptable control
306
performance using the model predictive control in this case.
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Table 5: Nonlinearity Index (this study) values for the selected system
Operating Ranges
Input Perturbation Magnitudes 0.05
0.10
0.15
0.20
SS-82
0.21
0.44
0.67
0.90
SS-83
0.22
0.48
0.75
1.03
SS-84
0.39
0.77
1.06
1.33
308 309
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Figure 5: Nonlinearity Index (this study) values for the selected system
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Table 6 and Figure 6 present the NM values for the system as the operating range moves
314
towards the azeotropic region. The NM value for operating range SS-83 with input magnitude
315
0.20 is less than 1, which suggests that the system can be considered linear in this range. This
316
value is also equal to the NM value for input magnitude 0.15, suggesting no increase in the
317
nonlinearity as the operating range is widened. However, the experimental observations in a
318
previous work have shown otherwise 55. Moreover, inconsistencies are observed as the NM for
319
operating range SS-84 with input magnitude 0.10 is less than that of 0.05 and for input
320
magnitude 0.20 is less than that of 0.15. Therefore, it can be concluded that the magnitude of
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NM is not able to track the actual nonlinearity of the system as the system moves near azeotropic
322
region.
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Table 6: Nonlinearity Measure (Du, 2017) values for the selected system Operating Ranges (mol%)
Input Perturbation Magnitudes 0.05
0.10
0.15
0.20
SS-82
0.48
0.59
0.77
0.82
SS-83
0.59
0.64
0.84
0.84
SS-84
1.07
0.88
2.67
1.63
325
326 327 328 329
Figure 6: Nonlinearity Measure (Du, 2017) values for the selected system Therefore, the values of the proposed NLI are more consistent and realistic in the prediction of the nonlinearity of the system than the previous observations of NM for the same system.
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4.3. FPE Comparison with NLI and NM To further establish the efficacy of the proposed index, the model residuals can be used as
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another criterion, since the nonlinearity of the system is also known as its inability to be
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represented effectively by a single linear model. The results in Table 7 and Figure 7 show that
335
the NLI values are more closely related to the observed logarithmic values of the FPE. The graph
336
shows that the NM values are continuously moving back and forth as the logarithmic values of
337
FPE increase. However, the NLI values are mostly showing a more predictable increase with the
338
increase in the logarithmic values of FPE. The adjusted R2 value for linear regression of NLI
339
against FPE is 0.84 whereas the adjusted R2 value for linear regression of NM against FPE is
340
only 0.40. Therefore, the NLI values are better representative of the nonlinearity of the system
341
than NM.
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Table 7: Comparison of NLI with NM with Model residuals log10 FPE
-10.7 -9.05 -7.94 -8.03 -8.78 -7.17 -5.95 -7.74 -6.63 -6.13 -5.28 -4.46
NLI
0.21
0.22
0.39
0.44
0.45
0.62
0.75
0.77
0.90
0.02
0.06
0.33
NM
0.48
0.59
1.07
0.59
0.64
0.75
0.84
0.88
0.88
0.88
2.67
1.63
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Figure 7: NLI and NM against FPE for the selected system
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4.4. Linear MPC Performance for different NLI values
347
In order to show how the system behaviour changes and control performance deteriorates as
348
the Nonlinearity index (NLI) values increase, a comparison is made for the setpoint tracking and
349
disturbance rejection performance of the operating regimes with different NLI values. The
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system was subjected to linear Model Predictive Control (MPC), which used the identified linear
351
model (Equation 12) for the selected operating ranges. The controller was appropriately tuned.
352
Setpoint changes were introduced as PRBS with magnitudes in accordance with the nonlinearity
353
index values of the system.
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Figure 8(a,b) show that the MPC is well-tuned for the control of the system and is able to track the set points and reject the disturbances in both positive and negative directions. From Figure 25 ACS Paragon Plus Environment
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8(a), it can be observed that the setpoint for the top composition is achieved within the first five
357
minutes of the change in setpoint, with an overshoot of 40%. Moreover, the system achieves the
358
setpoint for the bottom composition within the first fifteen minutes. In Figure 8(b) the
359
disturbance rejection is efficiently performed. The top and bottom compositions remain close to
360
the tolerance band.
361
These observations show that as the operating regime is mildly nonlinear i.e. has a low value
362
of NLI, the responses of the system are linear, and thus optimal input manipulations are carried
363
out for setpoint tracking and disturbance rejection. It can be concluded that the controller
364
performance of the system is satisfactory.
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(b) Disturbance Rejection – NLI = 0.65 Figure 8: Controller Performance (NLI=0.65)
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The setpoint tracking and disturbance rejection performance of the operating regime where the
371
system has just enough nonlinearity to be considered as nonlinear is presented in Figure 9(a,b). It
372
is observed that the tracking and rejection performances have just started to deteriorate, and the
373
controller action to achieve or maintain the setpoint has just started to be insufficient. Figure 9(a)
374
reveals that although the setpoints for the top composition are tracked within the first ten minutes
375
with only 35% overshoot, the response for bottom composition shows that a trade-off is being
376
made and the bottom composition is not being brought back to its reference point. The steady27 ACS Paragon Plus Environment
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state error, however, might be tolerable for some of the control applications where the tolerance
378
bands are wider. A similar behaviour is observed in the disturbance rejection plots i.e. Figure
379
9(b) where the disturbance is not completely rejected but is brought back near the tolerance band.
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Depending on the product specifications, some plant might tolerate the controller performance
381
of this magnitude. Nevertheless, it can be incurred that further widening of the operating regime
382
will result in poor setpoint tracking and rejection due to the increase in nonlinearity.
383 384
(a) Setpoint Tracking – NLI = 1.00
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(b) Disturbance Rejection – NLI = 1.00 Figure 9: Controller Performance (NLI=1.0) Figure 10(a,b) shows the setpoint tracking and disturbance rejection performance of the system
389
when the operating regime is wide enough to be significantly nonlinear (NLI=1.66). The NLI
390
magnitude suggests that the rejection and tracking should be poor, and the results confirm this
391
hypothesis. Large offsets are present, and the controller action is not able to track or maintain the
392
setpoint, thus poor controller performance is achieved.
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(a) Setpoint Tracking – NLI = 1.65
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(b) Disturbance Rejection – NLI = 1.65
397
Figure 10: Controller Performance (NLI=1.66)
398
4.5. Overall discussion
399
The efficacy of any proposed nonlinearity index depends on its ability to predict the behaviour
400
of the system with sufficient accuracy and consistency. The increased nonlinear behaviour of a
401
system, as well as the decline in the prediction accuracy and linear controller performance, are
402
used in this study as the outcomes of an increase in nonlinearity. The proposed nonlinearity
403
index is evaluated in such conditions and compared with another index proposed in the literature. 31 ACS Paragon Plus Environment
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These results clearly establish the superiority of the proposed NLI. Therefore, it can be
405
concluded that the system nonlinearity and behaviour is correctly predicted by the proposed NLI.
406
Importantly, the generic nature of this NLI can make it viable for the prediction of nonlinearity
407
for other control-relevant systems.
408
5. Conclusion
409
This study proposes an effective method to determine the extent of nonlinearity in the form of
410
the nonlinearity index (NLI). It is shown that the proposed nonlinearity index is able to estimate
411
the nonlinearity of system and is correlated to the linear model residuals and closed-loop model
412
predictive controller performance. The results are compared with the nonlinearity measure in
413
literature and observed that the proposed index is more consistent and relatable to the existing
414
results of the selected case study. Thus, the proposed NLI is an efficient and computation-
415
friendly index to evaluate the nonlinearity of systems. The index is generic in nature and can be
416
applied to other control-relevant systems.
417
6. Acknowledgements
418
The main author would like to thank Syed A. Taqvi for his valuable insights, comments and
419
suggestions used for the conceptualization and analysis of this study. The authors also recognize
420
the Graduate Assistance scheme provided by Universiti Teknologi PETRONAS for its
421
continuous support throughout the research.
422
7. References 32 ACS Paragon Plus Environment
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423 424 425 426 427
Industrial & Engineering Chemistry Research
1.
Hernjak, N.; Doyle, F. J., Correlation of process nonlinearity with closed-loop
disturbance rejection. Ind. Eng. Chem. Res 2003, 42 (20), 4611-4619. 2.
Xu, F.; Huang, B.; Akande, S., Performance assessment of model pedictive control for
variability and constraint tuning. Ind. Eng. Chem. Res 2007, 46 (4), 1208-1219. 3.
Nyström, R. H.; Böling, J. M.; Ramstedt, J. M.; Toivonen, H. T.; Häggblom, K. E.,
428
Application of robust and multimodel control methods to an ill-conditioned distillation column.
429
J. Process Control 2002, 12 (1), 39-53.
430 431 432 433 434
4.
Badwe, A. S.; Gudi, R. D.; Patwardhan, R. S.; Shah, S. L.; Patwardhan, S. C., Detection
of model-plant mismatch in MPC applications. J. Process Control 2009, 19 (8), 1305-1313. 5.
Uddin, F.; Tufa, L.; Yousif, S.; Maulud, A., Comparison of ARX and ARMAX
Decorrelation Models for Detecting Model-Plant Mismatch. Procedia Eng. 2016, 148, 985-991. 6.
Yao, J.-Y.; Lin, S.-Y.; Chien, I. L., Operation and control of batch extractive distillation
435
for the separation of mixtures with minimum-boiling azeotrope. J. Chin. Inst. Chem. Eng, 2007,
436
38 (5-6), 371-383.
437 438 439 440 441 442
7.
Huang, H. J.; Chien, I. L., Choice of suitable entrainer in heteroazeotropic batch
distillation system for acetic acid dehydration. J. Chin. Inst. Chem. Eng, 2008, 39 (5), 503-517. 8.
Taqvi, S. A.; Tufa, L. D.; Mahadzir, S., Optimization and Dynamics of Distillation
Column Using Aspen Plus®. Procedia Eng. 2016, 148, 978–984. 9.
Luyben, W. L., Rigorous dynamic models for distillation safety analysis. Comput. Chem.
Eng. 2012, 40, 110-116. 33 ACS Paragon Plus Environment
Industrial & Engineering Chemistry Research 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60
443 444
10. Luyben, W. L., Distillation design and control using Aspen simulation. John Wiley & Sons: 2013.
445
11. Taqvi, S. A.; Tufa, L. D.; Zabiri, H.; Mahadzir, S.; Maulud, A. S.; Uddin, F., Rigorous
446
dynamic modelling and identification of distillation column using Aspen Plus. 2017, 262-267.
447 448
12. Beale, E. M. L., Confidence Regions in Non-Linear Estimation. J. R. Stat. Soc. Series B Stat. Methodol. 1960, 42 (1), 41-88.
449
13. Bucci, O. M.; Cardace, N.; Crocco, L.; Isernia, T., Degree of nonlinearity and a new
450
solution procedure in scalar two-dimensional inverse scattering problems. J. Opt. Soc. Am. A
451
2001, 18 (8), 1832.
452 453 454 455 456 457 458 459 460 461
14. Desoer, C.; Yung-Terng, W., Foundations of feedback theory for nonlinear dynamical systems. IEEE Transactions on Circuits and Systems 1980, 27 (2), 104-123. 15. Nikolaou, M. When is Nonlinear Dynamic Modeling Necessary?, Amer. Contr. Conf., IEEE: 1993. 16. Emancipator, K.; Kroll, M. H., A quantitative measure of nonlinearity. Clin. Chem. 1993, 39 (5), 766-72. 17. Yoshida, H.; Komai, M.; Yana, K., An index of system nonlinearity and its estimation. Proc. - Int. Conf. Neural Networks 1993, 2, 2021-2024. 18. Mizuta, H.; Jibu, M.; Yana, K., Adaptive estimation of the degree of system nonlinearity. Proc. - IEEE Adapt. Sys. Signal Process. Comm. Control Symp. 2000, 352-356.
34 ACS Paragon Plus Environment
Page 34 of 41
Page 35 of 41 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60
462 463 464 465 466 467 468 469 470 471 472 473 474 475 476 477 478
Industrial & Engineering Chemistry Research
19. Helbig, A.; Marquardt, W.; Allgöwer, F., Nonlinearity measures: definition, computation and applications. J. Process Control 2000, 10 (2-3), 113-123. 20. Harris, K. R.; Colantonio, M. C.; Palazoğlu, A., On the computation of a nonlinearity measure using functional expansions. Chem. Eng. Sci. 2000, 55 (13), 2393-2400. 21. Hahn, J.; Edgar, T. F., A gramian based approach to nonlinearity quantification and model classification. Ind. Eng. Chem. Res 2001, 40 (24), 5724-5731. 22. Sun, D.; Hoo, K. A., Non-linearity measures for a class of SISO non-linear systems. Int. J. Control 2000, 73 (1), 29-37. 23. Liu, Y.; Li, X. R., Measure of Nonlinearity for Estimation. IEEE Trans. Signal Process. 2015, 63 (9), 2377-2388. 24. El-Sakkary, A., The gap metric: Robustness of stabilization of feedback systems. IEEE Trans. Autom. Control 1985, 30 (3), 240-247. 25. Georgiou, T. T.; Smith, M. C., Optimal robustness in the gap metric. IEEE Trans. Autom. Control 1990, 35 (6), 673-686. 26. Tan, W.; Marquez, H. J.; Chen, T.; Liu, J., Analysis and control of a nonlinear boilerturbine unit. J. Process Control 2005, 15 (8), 883-891. 27. Galán, O.; Romagnoli, J. A.; Palazoǧlu, A.; Arkun, Y., Gap metric concept and
479
implications for multilinear model-based controller design. Ind. Eng. Chem. Res 2003, 42 (10),
480
2189-2197.
35 ACS Paragon Plus Environment
Industrial & Engineering Chemistry Research 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60
481 482 483 484
28. Kuure-Kinsey, M.; Bequette, B. W., Multiple model predictive control strategy for disturbance rejection. Ind. Eng. Chem. Res 2010, 49 (17), 7983-7989. 29. Arslan, E.; Çamurdan, M. C.; Palazoglu, A.; Arkun, Y., Multimodel scheduling control of nonlinear systems using gap metric. Ind. Eng. Chem. Res 2004, 43 (26), 8275-8283.
485
30. Du, J.; Song, C.; Li, P., Multimodel control of nonlinear systems: an integrated design
486
procedure based on gap metric and H∞ loop shaping. Ind. Eng. Chem. Res 2012, 51 (9), 3722-
487
3731.
488 489 490 491 492
31. Du, J.; Johansen, T. A., Integrated multimodel control of nonlinear systems based on gap metric and stability margin. Ind. Eng. Chem. Res 2014, 53 (24), 10206-10215. 32. Du, J.; Johansen, T. A., Integrated multilinear model predictive control of nonlinear systems based on gap metric. Ind. Eng. Chem. Res 2015, 54 (22), 6002-6011. 33. Tao, X.; Li, D.; Wang, Y.; Li, N.; Li, S., Gap-metric-based multiple-model Predictive
493
control with a polyhedral stability region. Ind. Eng. Chem. Res 2015, 54 (45), 11319-11329.
494
34. Guay, M.; Dier, R.; Hahn, J.; McLellan, P., Effect of process nonlinearity on linear
495 496 497 498 499
quadratic regulator performance. J. Process Control 2005, 15 (1), 113-124. 35. Guay, M., The effect of process nonlinearity on linear controller performance in discretetime systems. Comput. Chem. Eng. 2006, 30 (3), 381-391. 36. Guay, M.; Forbes, J. F., On the Effect of Non‐Linearity on Linear Quadratic Regulator Stability and Performance. Can. J. Chem. Eng. 2007, 85 (1), 101-110.
36 ACS Paragon Plus Environment
Page 36 of 41
Page 37 of 41 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60
500 501 502 503 504
Industrial & Engineering Chemistry Research
37. Li, J.; Tan, W.; Fu, C. In Nonlinearity measure based on disturbance rejection, Chin. Control Decis. Conf., IEEE: 2009; pp 3487-3492. 38. Liu, J.; Meng, Q.; Fang, F., Minimum variance lower bound ratio based nonlinearity measure for closed loop systems. J. Process Control 2013, 23 (8), 1097-1107. 39. Bates, D. M.; Watts, D. G., Nonlinear Regression: Iterative Estimation and Linear
505
Approximations. In Nonlinear Regression Analysis and Its Applications, Bates, D. M.; Watts, D.
506
G., Eds. Wiley Inc.: 2008; pp 32-66.
507 508
40. Bates, D. M.; Watts, D. G., Relative Curvature Measures of Nonlinearity. J. R. Stat. Soc. Series B Stat. Methodol. 1980, 42 (1), 1-25.
509
41. Bates, D. M.; Hamilton, D. C.; Watts, D. G., Calculation of intrinsic and parameter-
510
effects curvatures for nonlinear regression models. Commun Stat Simul Comput. 2007, 12 (4),
511
469-477.
512
42. Drummond, O. E.; La Scala, B. F.; Mallick, M.; Arulampalam, S.; Teichgraeber, R. D.,
513
Differential geometry measures of nonlinearity for filtering with nonlinear dynamic and linear
514
measurement models. Signal Data Process. Small Targets 2007, 6699.
515
43. Niu, R.; Varshney, P. K.; Alford, M.; Bubalo, A.; Jones, E.; Scalzo, M., Curvature
516
nonlinearity measure and filter divergence detector for nonlinear tracking problems. In 11th Int.
517
Conf. Inf. Fusion, 2008; pp 1-8.
518
44. Mallick, M.; Scala, B. F. L.; Arulampalam, M. S. Differential geometry measures of
519
nonlinearity for the bearing-only tracking problem, Defense and Security, SPIE: 2005; p 13. 37 ACS Paragon Plus Environment
Industrial & Engineering Chemistry Research 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60
520 521
45. Mallick, M.; la Scala, B. F., Differential Geometry Measures of Nonlinearity for Ground Moving Target Indicator (GMTI) Filtering. In 7th Int. Conf. Inf. Fusion, 2005, 219-226.
522
46. Mallick, M.; Arulampalam, S.; Yanjun, Y.; Mallick, A., Connection between differential
523
geometry and estimation theory for polynomial nonlinearity in 2D. In 13th Int. Conf. Inf. Fusion,
524
2010, 1-8.
525 526 527
47. Fuxman, A.; Forbes, F.; Hayes, R. Measure of nonlinearity for hyperbolic distributed parameter systems, In Eur. Conf. Control, IEEE: 2007; pp 5580-5586. 48. Mandic, D. P.; Vayanos, P.; Javidi, S.; Jelfs, B.; Aihara, K., Online tracking of the degree
528
of nonlinearity within complex signals. IEEE Trans. Acoust., Speech, Signal Process. 2008,
529
2061-2064.
530 531 532 533 534 535 536 537 538 539
49. Haber, R., Nonlinearity Tests for Dynamic Processes. IFAC Proc. Vol. 1985, 18 (5), 409414. 50. Billings, S. A.; Voon, W. S. F., Correlation based model validity tests for non-linear models. Int. J. Control 1986, 44 (1), 235-244. 51. Tugnait, J. K., Testing for linearity of noisy stationary signals. IEEE Transactions on Signal Processing 1994, 42 (10), 2742-2748. 52. Schreiber, T., Interdisciplinary application of nonlinear time series methods. Phys. Rep. 1999, 308 (1), 1-64. 53. Schreiber, T.; Schmitz, A., Discrimination power of measures for nonlinearity in a time series. Phys. Rev. E 1997, 55 (5), 5443. 38 ACS Paragon Plus Environment
Page 38 of 41
Page 39 of 41 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60
540 541 542
Industrial & Engineering Chemistry Research
54. Barnett, A. G.; Wolff, R. C., A time-domain test for some types of nonlinearity. IEEE Trans. Signal Process. 2005, 53 (1), 26-33. 55. Uddin, F.; Tufa, L. D.; Shah Maulud, A.; Taqvi, S. A., System Behavior and Predictive
543
Controller Performance Near the Azeotropic Region. Chem. Eng. Technol. 2018, 41 (4), 806-
544
818.
545 546 547 548
56. Taqvi, S. A.; Tufa, L. D.; Mahadzir, S., Rigorous Steady-State Simulation of Acetone Production using Aspen HYSYS®. Aust. J. Basic Appl. Sci. 2016, 9 (36), 535-542. 57. Taqvi, S. A.; Tufa, L. D.; Zabiri, H.; Maulud, A. S.; Uddin, F., Fault detection in distillation column using NARX neural network. Neural Comput. Appl. 2018, 1-17.
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58. Uddin, F.; Tufa, L. D.; Taqvi, S. A.; Vellen, N., Development of Regression Models by
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Closed–Loop Identification of Distillation Column - A Case Study. Indian J. Sci. Technol. 2017,
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10 (2).
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59. Du, J.; Johansen, T. A., Control-relevant nonlinearity measure and integrated multimodel control. J. Process Control 2017, 57, 127-139.
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Author Contributions
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The manuscript was written through equal contributions of all authors. All authors have given approval to the final version of the manuscript.
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ABBREVIATIONS
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NLI, Nonlinearity Index; MIMO, Multiple-Input-Multiple-Output; NM, Nonlinearity Measure; MPC, Model Predictive Control; RG, Relative Gain; FPE, Final Prediction Error; MSE, Mean Square Error; FOPTD, first order plus time delay; MPM, model-plant mismatch; LQG, linear 39 ACS Paragon Plus Environment
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quadratic gaussian; P, Proportional; PI, Proportional-Integral; PID, Proportional-IntegralDerivative; PRBS, Pseudo Random Binary Signal.
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