and analytical applications in a future p u b l i c a t i o n (12).
Acknowledgment I extend my gratitude to a number of m y f r i e n d s a n d c o l l e a g u e s w i t h w h o m I have collaborated in C A R S o v e r t h e p a s t s e v e r a l y e a r s . T h e s e inc l u d e R. B y e r , S. H a r r i s , a n d R. B e gley ( f o r m e r l y ) a t S t a n f o r d ; G. K l a u minzer at Molectron Corp., J.-P. T a r a n a t O N E R A in F r a n c e ; R. D e W i t t , W . S h a u b , S. L e m o n t , R . Gammon, and J. McDonald a t NRL; W. Sanders (Catholic University); W. Toiles a t the Naval Postgraduate School; a n d especially J. Nibler (Oregon S t a t e University) w h o s p e n t a very productive sabbatical year a t N R L . I a l s o t h a n k L. C a r r e i r a a n d L . G o s s ( U n i v e r s i t y of G e o r g i a ) for allowing m e t o i l l u s t r a t e t h e i r s p e c t r a p r i o r to publication.
References (1) N. Bloemhergen, "Nonlinear Optics", Benjamin, Reading, Mass., 1965; C. Flynzanis, "Quantum Electronics—A Treatise", H. Rabin and C. Tang, Eds., Vol 1, Academic Press, New York, N.Y., 1975; F. Zernike and J. E. Midwinter, "Applied Nonlinear Optics", Wiley, New York, N.Y., 1973; A. Yariv, "Introduction to Quantum Electronics", 2nd éd., Wiley, New York, N.Y., 1975.
(2) R. L. Byer and R. L. Herbert, " P a r a metric Oscillation and Mixing", in "Nonlinear Infrared Generation", Y.-R. Shen, Ed., p 81, Springer-Verlag, Berlin, Germany, 1977. (3) J. Reinjes et al., Appl. Phys. Lett., 30, 480(1977). (4) W. M. Toiles, -I. W. Nibler, J. R. McDonald, and A. B. Harvey, Appl. Spectrosc, 3 1 , 253 (1977); J. W. Nibler, W. M. Shaub, J. R. McDonald, and A. B. Harvey, "Coherent Anti-Stokes Raman Spectroscopy", in "Vibrational Spectra and Structure", J. R. Durig, Ed., Vol 6, Elsevier, New York, N.Y., 1977; J. W. Nibler and A. B. Harvey, "Applications of CARS", in "Analytical Raman Spectroscopy", W. Keifer, Ed., Wiley-Interscience, New York, N.Y., 1977; A. B. Harvey and J. W. Nibler, Appl. Spectrosc. Rev., in press (1978); J. W. Nibler and G. V. Knighten, "Coherent AntiStokes Raman Spectroscopy", in "Topics in Applied Physics", A. Weber, Ed., Chap. 7, Springer-Verlag, 1977; H. C. Andersen and B. S. Hudson, "Coherent Anti-Stokes Raman Scattering", in "Molecular Spectroscopy", D. A. Long, Ed., Vol 5, Chemical Society, London, England, 1977. (5) N. B. Colthup, L. H. Daly, and S. E. Wiberly, "Introduction to Infrared and Raman Spectroscopy", 2nd éd., Academic Press, New York, N.Y., 1975. (6) R. N. DeWitt, A. B. Harvey, and W. M. Toiles, "Theoretical Development of Third-Order Susceptibility as Related to Coherent Anti-Stokes Raman Spectroscopy (CARS)", N R L Memorandum Report 3260, April 1976; Ret. (4a) and references therein. (7) B. S. Hudson, Ann. Rev. Biophys. Biocng., 6, 135(1977).
(8) L. A. Carreira and L. P. Goss, in press. (9) J. W. Nibler, J. R. McDonald, and A. B. Harvey, Opt. Commun., 18, 371 (1976); W. M. Shaub, J. W. Nibler, and A. B. Harvey, J. Chem. Phys., 67, 1883 (1977). (10) W. B. Roh, P. Schreiber, and J.-P.E. Taran, Appl. Phys. Lett., 29, 174 (1976); W. B. Roh and P. W. Schreiber, Appl. Opt., 17, xx (1978). (11) M. R. Aliev, D. N. Kozlov, and V. V. Smirnov, JETP Lett., 26,31 (1977). (12) A. B. Harvey, Ed., "Chemical Applications of Nonlinear Spectroscopy", Academic Press, to be published in 1979.
Albert B. Harvey is head of the Naval Research Laboratory's Chemical Diagnostics Branch. His research interests include optical diagnostics of chemical systems, kinetics of gas phase reactions, chemical lasers and energy transfer, and novel methods of trace analysis and control.
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