Article pubs.acs.org/JPCA
Principles and Applications of Broadband Impulsive Vibrational Spectroscopy M. Liebel,† C. Schnedermann, T. Wende, and P. Kukura*
Downloaded by WEST VIRGINIA UNIV on September 10, 2015 | http://pubs.acs.org Publication Date (Web): August 31, 2015 | doi: 10.1021/acs.jpca.5b05948
Physical and Theoretical Chemistry Laboratory, University of Oxford, South Parks Road, OX1 3QZ Oxford, U.K. ABSTRACT: We present an experimental setup for recording vibrational coherences and thereby Raman spectra of molecules in their ground and excited electronic states over the 50−3000 cm−1 spectral range using broadband impulsive vibrational spectroscopy. Our approach relies on the combination of a
