Quantized Conduction and High Mobility in ... - ACS Publications

Sep 20, 2015 - Cezar B. Zota,*,† David Lindgren,‡ Lars-Erik Wernersson,† and Erik Lind†. †. Department of Electrical and Information Technol...
1 downloads 0 Views 1MB Size
Subscriber access provided by University of Otago Library

Article

Quantized Conduction and High Mobility in Selectively Grown InGa As Nanowires x

1-x

Cezar B. Zota, David Lindgren, Lars-Erik Wernersson, and Erik Lind ACS Nano, Just Accepted Manuscript • DOI: 10.1021/acsnano.5b03318 • Publication Date (Web): 20 Sep 2015 Downloaded from http://pubs.acs.org on September 23, 2015

Just Accepted “Just Accepted” manuscripts have been peer-reviewed and accepted for publication. They are posted online prior to technical editing, formatting for publication and author proofing. The American Chemical Society provides “Just Accepted” as a free service to the research community to expedite the dissemination of scientific material as soon as possible after acceptance. “Just Accepted” manuscripts appear in full in PDF format accompanied by an HTML abstract. “Just Accepted” manuscripts have been fully peer reviewed, but should not be considered the official version of record. They are accessible to all readers and citable by the Digital Object Identifier (DOI®). “Just Accepted” is an optional service offered to authors. Therefore, the “Just Accepted” Web site may not include all articles that will be published in the journal. After a manuscript is technically edited and formatted, it will be removed from the “Just Accepted” Web site and published as an ASAP article. Note that technical editing may introduce minor changes to the manuscript text and/or graphics which could affect content, and all legal disclaimers and ethical guidelines that apply to the journal pertain. ACS cannot be held responsible for errors or consequences arising from the use of information contained in these “Just Accepted” manuscripts.

ACS Nano is published by the American Chemical Society. 1155 Sixteenth Street N.W., Washington, DC 20036 Published by American Chemical Society. Copyright © American Chemical Society. However, no copyright claim is made to original U.S. Government works, or works produced by employees of any Commonwealth realm Crown government in the course of their duties.

Page 1 of 25

1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60

ACS Nano

Quantized Conduction and High Mobility in Selectively Grown InxGa1-xAs Nanowires Cezar B. Zota,*,† David Lindgren,§ Lars-Erik Wernersson† and Erik Lind† †

Department of Electrical and Information Technology, Lund University, Box 118, 22100 Lund,

Sweden. §

Division of Solid State Physics, Lund University, Box 118, 22100 Lund, Sweden

KEYWORDS Field effect transistors, nanowire, electric transport, mobility, InGaAs, ballistic transport, selective regrowth, photoluminescence, Raman

ABSTRACT

We report on measured quantized conductance and quasi-ballistic transport in selectively regrown In0.85Ga0.15As nanowires. Very low parasitic resistances obtained by regrowth techniques allow us to probe the near-intrinsic electrical properties, and we observe several quantized conductance steps at 10 K. We extract a mean free path of 180 ± 40 nm and an

ACS Paragon Plus Environment

1

ACS Nano

1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60

Page 2 of 25

effective electron mobility of 3300 ± 300 cm2/V⋅s, both at room-temperature, which are among the largest reported values for nanowires of similar dimensions. In addition, optical characterization of the nanowires by photoluminescence and Raman measurement is performed. We find an unintentional increase of Indium in the InxGa1-xAs composition relative the regrown film layer, as well as partial strain relaxation.

Indium-rich InxGa1-xAs nanowires have gathered much recent research attention due to their excellent electron transport properties.1 In particular, InAs nanowires have been shown to have least an order of magnitude higher mobility than Silicon nanowires.2,3 Moreover, the ease by which ohmic contacts are formed to InxGa1-xAs, and the possibility of low-defect high-k oxides interfaces, has made InxGa1-xAs one of the primary considerations as the replacement for Silicon channels in n-type metal-oxide-semiconductor field effect transistors (MOSFETs).4–7 The implementation of III-V MOSFETs such as InxGa1-xAs will likely be in the form of 1D nanowires with diameters below 30 nm.8 The use of nanowires as the channel in MOSFETs offers enhanced performance compared to traditional planar channels, through improved electrostatic control. The combination of high-mobility materials and the short gate-lengths (~30 nm) of state-of-the-art MOSFETs indicate operation in the ballistic or quasi-ballistic regime. Together with 1D channels, such devices display unique characteristics, notably quantized conduction, step-like features in the conductance at low temperatures. Several methods of fabricating InxGa1-xAs nanowires have been reported. In particular, nanowires grown by the vapor-liquid-solid (VLS) technique, employing a metal particle catalyst, have been widely studied.9 VLS-grown InAs nanowires, for instance, exhibit mobility ranging

ACS Paragon Plus Environment

2

Page 3 of 25

1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60

ACS Nano

from 2000 to 5000 cm2/Vs at nanowire diameters of