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Characterization of Natural and Affected Environments
Nighttime light images reveal spatial-temporal dynamics of global anthropogenic resources accumulation above ground Bailang Yu, Shunqiang Deng, Gang Liu, Chengshu Yang, Zuoqi Chen, Catherine Jane Hill, and Jianping Wu Environ. Sci. Technol., Just Accepted Manuscript • DOI: 10.1021/acs.est.8b02838 • Publication Date (Web): 12 Sep 2018 Downloaded from http://pubs.acs.org on September 19, 2018
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Nighttime light images reveal spatial-temporal dynamics of global
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anthropogenic resources accumulation above ground
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Bailang Yu 1,2, Shunqiang Deng 1,2, Gang Liu
4
*, 3
, Chengshu Yang 1,2, Zuoqi Chen 1,2,
Catherine Jane Hill 3, Jianping Wu 1,2
5 6 7
1
8
China Normal University, Shanghai 200241, China;
9
2
Key Laboratory of Geographic Information Science, Ministry of Education, East
School of Geographic Sciences, East China Normal University, Shanghai 200241,
10
China;
11
3
12
and Environmental Technology, University of Southern Denmark, 5230 Odense,
13
Denmark.
14
TOC Art
SDU Life Cycle Engineering, Department of Chemical Engineering, Biotechnology,
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ABSTRACT
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Urbanization and industrialization represent largely a process of transforming
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materials from biosphere and lithosphere to anthroposphere. Understanding the
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patterns of such anthropogenic material stock accumulation is thus a fundamental
21
prerequisite to assess and sustain how humans alter the biophysical movements of
22
resources around Earth. Previous studies on these anthropogenic stocks, however, are
23
often limited to the global and national scales, due to data gaps at higher spatial
24
resolutions. Here, based on a new set of national materials stock data and nighttime
25
light images, we developed a regression model to map the global anthropogenic
26
stocks of three fundamental construction materials (steel, concrete, and aluminium) at
27
a 1 km×1 km level from 1992 to 2008. We revealed an unevenly distributed pattern,
28
with over 40% found in three belts: from England across the Channel to Western
29
Europe; from eastern coast China to South Korea and Japan; and from Great Lakes
30
along eastern coast of United States to Florida. The spatial-temporal dynamics of
31
global anthropogenic stocks at smaller spatial scales reflect a combined effect of
32
physical geography, architectural and construction specifications, and socioeconomic
33
development. Our results provide useful data that can potentially support
34
policy-makers and industry on resource efficiency, waste management, urban mining,
35
spatial planning, and environmental sustainability at regional and urban scales.
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1. INTRODUCTION
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Human civilization is built upon the use of natural resources. Industrialization and
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urbanization in the past centuries have been transforming vast amount of raw
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materials from biosphere and lithosphere to human built-environment1,2. Such a
41
continuing use of raw materials has raised concerns on both growing resource scarcity
42
and supply constraint3 and increasing environmental challenges (e.g., climate change4)
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associated with materials production and consumption. The understanding of these
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patterns of materials use is thus a fundamental prerequisite to explore pathways
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towards a sustainable materials management and strategies for environmental impacts
46
mitigation.
47 48
Many previous efforts5,6 have been devoted to characterizing the patterns of global
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and national material flows and developing indicators to inform relevant resource
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policy. For example, EU member states have started to compile economic-wide
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material flow accounts (e.g., domestic material extraction and total material
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requirement) since 20077. The patterns of the accumulation of these materials in our
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societies (e.g., buildings, infrastructure, and consumer goods), often referred as in-use
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stocks, built environment stocks, or anthropogenic stocks (which is used consistently
55
hereafter in this paper), however, are less understood comparing to flows. These
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anthropogenic stocks are important for ensuring both human development and
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environmental sustainability because: (i) They are actively used by households,
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governments, the public, or industries, over years and decades to satisfy service
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demand (e.g., shelter and transportation) and to facilitate industrial production8–10; (ii)
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They set boundary conditions for upstream raw materials demand and availability of
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secondary materials at their end of life that can be recovered through urban mining4,11;
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and (iii) They shape the physical setting of our economy and society and thus have
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lock-in effects on societal energy use and emissions both directly (the operation of
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stocks, e.g., fuel consumption of cars) and indirectly (the construction of stocks, e.g.,
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energy use of cement production)4,10.
66 67
Existing studies on the characterization of anthropogenic stocks deploy either a
68
top-down approach or a bottom-up approach12. With a top-down approach, the
69
historical consumption of materials in different applications (e.g., buildings and
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transportation) and their corresponding lifetime are used to simulate the
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anthropogenic stocks. Case studies include metals such as iron and steel13, copper14,
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aluminum11, and rare earth elements15 and nonmetal materials such as cement16 and
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carbon17. However, this approach is practically limited to a global or national level
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due to data gaps (e.g., trade data or apparent consumption data often not available on
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the regional level) and lacks a spatial resolution. The estimation of initial stock can be
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a challenge too especially for products with long life time like buildings and
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infrastructure18. This might be complemented by a bottom-up approach, with which
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all the relevant goods in a city or region and their corresponding material composition
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are counted and then aggregated. However, these studies are usually very data and
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labor intensive and depend highly on statistics, and thus usually cover only very few
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case cities19,20 or countries18,21 and years21.
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Recently, the satellite and remote sensing data and techniques are increasingly applied
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in socio-economic indicators22,23 and urban characteristics studies24, and open a new
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window for the estimation of geographically refined materials stock. For example,
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nighttime lights images are found to correlate well with anthropogenic material stocks
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and thus regression models are used to disaggregate anthropogenic stocks on the
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country level to a more refined level25–28. However, these attempts often lack a good
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basis of stock estimation on the country level and use only one or a few reported
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values as a starting point in the regression. For example, Rauch27 used only some 6-16
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samples of anthropogenic metal stock on the country level as a basis to simulate
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stocks of other countries using their correlation with gross domestic product (GDP).
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These results are also mostly for static years27,28 and selected sectors and materials
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(predominately for steel26,29), and thus could not inform temporal trends and include
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other important building materials such as concrete and aluminum.
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Here, based on a new set of anthropogenic material stocks data for all world countries
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in the past decades and a generated long-term dataset of nighttime lights images
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obtained by the Defense Meteorological Satellite Programs’ Operational Line-scan
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System (DMSP/OLS), we show to date the most comprehensive global mapping of
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anthropogenic stocks (using the three key construction materials, cement, steel, and
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aluminum, as a proxy) by 1km-1km grids from 1992 to 2008. We then discuss drivers
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behind the spatial-temporal dynamics of global anthropogenic stocks at smaller spatial
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scales and implications on resource efficiency, waste management, urban mining,
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spatial planning, and environmental sustainability.
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2. MATERIALS AND METHODS
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2.1 National anthropogenic stocks of aluminum, cement, and steel. We used data
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in our earlier studies and other literature for national anthropogenic stocks of cement
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(1992-2009; or cement equivalent in concrete)16, steel (1992-2008)30, and aluminum
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(1992-2010)11 for over 130 world countries or regions in the past decades. These data
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were generated based on a top-down approach as briefly described as follows (more
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methodology details can be found in our earlier studies11,16): For each material, its
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cycle from production to use and end-of-life management was simulated and all
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relevant anthropogenic stocks and flows within the cycle were quantified. Starting
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points were either production or domestic shipment, which were further adjusted by
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international trade flows of materials in semis and final products to calculate the flows
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entering the use phase. Different end-use categories (such as buildings and
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constructions, transportation, machinery and equipment, and packaging) were
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considered and their corresponding lifetimes following a normal distribution were
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assumed and differentiated by category and by country to simulate the flows exiting
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from the use phase and eventually the anthropogenic stocks accumulated.
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2.2 Preprocessing of multi-temporal datasets of nighttime light data. Acquired
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from the National Geophysical Data Center (NGDC) of NOAA
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(http://ngdc.noaa.gov/eog/), satellite imageries of DMSP/OLS Nighttime Stable
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Lights (NSL) Time Series (Version 4) applied in this study cover a 19-year timespan
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from 1992 to 2010 and almost the whole globe. The images are obtained from six
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individual satellites (F10, F12, F14, F15, and F16) of various periods and they are
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annually composited. With digital number (DN) values of 0∼63 and spatial resolution
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of 30 arc seconds (∼ 1km), the NSL data record light frequency on specifically
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observed pixels. Since the DMSP/OLS sensor has no in-flight calibration, the original
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composites of different satellites cannot be compared directly.
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A saturated correction was considered because the range of the data is limited to 0∼63
136
and cannot express even higher light intensity, so we performed inter calibration and
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saturated correction to build up a comparable time series of nighttime light data based
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on a dependable image registration approach named invariant target method31.
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Specifically, we first identified an invariant region (Hegang city, China, in this case)
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where light intensity was stable during the whole study period. Then we chose the
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DMSP/OLS image of year 2006 as a reference and built a power function model using
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pixels of Hegang city as samples. In the end, we estimated the coefficients and
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applied the model to the whole image to have saturated pixels corrected. This inter
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calibrated method may lead to uncertainty and gaps between the start year and the end
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year and their adjacent years because they do not have any year to refer to.
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As anthropogenic stocks are mainly found in buildings and infrastructure, especially
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common seen in urban areas, we implemented a natural-city extraction method
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proposed by Jiang32 to limit the estimated anthropogenic stocks inner urban area and
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set light intensity outside natural city regions to zero. Using zonal statistics method
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provided by ArcGIS, values of a nighttime light image for all natural city areas inner a
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specific country or region are summarized as the indicator of light intensity for that
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country or region, so that a corresponding dataset of light intensity and anthropogenic
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stocks on the country level can be generated to conduct the regression models.
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2.3 Development of regression models between anthropogenic stocks and
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nighttime light intensity. Both anthropogenic stocks and nighttime light data are
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indicators of anthropogenic activities. Previous studies have shown that nighttime
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lights correlate relatively well with social-economic indicators such as GDP27,
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regional population33, electricity consumption34, and carbon emissions35 by either
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linear regression models or double-log models. In this study, we assumed that an
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empirical power function is appropriate, as suggested by previous studies26, to
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describe the relationship between anthropogenic stocks and nighttime light data:
= ℎ ∗ 164
(1)
Which can be transformed to double-log form as:
log = + ∗ log ℎ
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(2)
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Where stock and light represent corresponding mass of anthropogenic stocks and
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intensity of nighttime light locally, and , are coefficients of the regression model.
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Since the absolute quantity of national anthropogenic stocks is of great difference due
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to individual heterogeneity, we normalized the anthropogenic stocks and nighttime
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light data by total natural city area of each country or region. Thus the model can be
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revised as:
ln__ = + ∗ ln ℎ__
(3)
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Where __ and ℎ__ are stocks mass and light intensity in
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an unit area (1km * 1km grid). For each type of anthropogenic stocks and every year
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in the given time ranges, we are able to build a simple double-log regression model.
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Figure 1. Scatterplot of the relationship between anthropogenic steel stocks and
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nighttime light intensity for the year 2008. For scatterplots of all materials and all
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years, see section 1.1, Figure S1-S54, in the Supporting Information.
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Figure 1 is a case of relationships between anthropogenic steel stocks and nighttime
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light intensity for the year 2008. To avoid potential influence of outliers, a
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density-based spatial clustering of applications with noise (DBSCAN) is implemented
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and some outlier points are consequently removed. Using an ordinary least square
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estimator we get a strong correlation with R2 = 0.90 under 20 test samples. Similarly,
184
we can generate regression models for each year and each construction material to
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describe the relationship between anthropogenic stocks and nighttime light intensity,
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and the coefficients of the models are all significant at a 95% confidence (see details
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in Tables S1-S3 in the Supporting Information).
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2.4 Model applications and gridded anthropogenic stocks. Applying the simple
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double-log linear regressions represented above, we were able to estimate the
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parameters by country and by material given in the models, and thus, calculate the
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quantity of anthropogenic stocks at a 1km grid level per country per year. For the
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convenience of visualization at a sub-country level, we adopted boundary line data of
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cities from the Database of Global Administrative Areas (GADM; https://gadm.org/),
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which may be slightly different from data from statistics.
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3. RESULTS AND DISCUSSION
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3.1 Spatial-temporal dynamics of anthropogenic stocks at different geographical
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levels. We found that material stocks are widely distributed in human settlements
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across the world (Figure 2), and rapid industrialization36 and massive urbanization37 in
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the past decades have absorbed vast amount of construction materials into buildings
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and infrastructure. The global anthropogenic stocks have doubled in two decades from
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about 36.3 billion tons in 1992 to over 75.4 million tons in 2008. Figure 2 also shows
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that global anthropogenic stocks are not evenly distributed, ranging from averagely
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about 26,000 tons/km2 in Africa to 38,000 tons/km2 in Asia to over 40,000 tons/km2
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in Europe, America, and Oceania. Three regions or belts possess over 40% of global
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anthropogenic stocks in 2008: (1) Most of Europe, from England across the Channel
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to Germany, southern to Italy and Spain; (2) East Asia, from eastern coast China to
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South Korea and Japan; (3) East and northeastern United States, along Great Lakes
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and eastern coast to Florida. These identified regions are in general consistent with
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results of Rauch27 for the world’s anthropogenic stock of four metals (iron, aluminium,
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copper, and zinc) in 2000.
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At the country level, it can be seen that the North China Plain, the Yangtze River
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Delta, and the Pearl River Delta of China, where drastic urbanization is taking
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place37,38, have become clearly most important anthropogenic stocks deposits, while
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western Europe, the main island of Japan, and eastern United States shows a relatively
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more even distribution due to its steady urbanization and economic growth. New
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York metropolitan regions have the world’s highest anthropogenic stocks density (up
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to approximately 59,000 tons/km2 on average), due to its dense population and
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crowded skyscrapers. In addition, a few other world regions also possess large
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quantity of anthropogenic stocks, such as regions around Johannesburg, Rio de
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Janeiro, the Nile Valley, west bank of the Persian Gulf, and the north side of Malacca,
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where there are important seaports, estuary, or regional central cities.
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Figure 2. Global mapping of anthropogenic stocks (adding up cement, steel, and aluminum) in 2008 (tons/km2) at a 1 km1 km grid level. a) Part of Europe and North Africa; b) East Asia (eastern China, South Korea, and Japan); c) North America (mainly USA and southern Canada). Figures for specific materials can be found in the Supplementary Information (Section 1 Figure S55-S125).
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We visualized the varying temporal dynamics of anthropogenic stocks at smaller
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spatial scales in different regions in Figure 3, based on RGB (with red, green, and
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blue representing the total anthropogenic stocks in 1992, 2000, and 2008, respectively)
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composite images.
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•
In Figure 3a, for example, southern Europe is dominated by white and is of greater
231
brightness than North Africa, indicating a steady yet overall larger amount of
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anthropogenic stocks in the long run (fluctuating between 48,000 tons/km2 and
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52,000 tons/km2). On the contrary, North Africa shows more blue areas, indicating
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a relatively lower (about 23,000 tons/km2) but increasing pattern of anthropogenic
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stocks accumulation between 2000 and 2008. This manifests the rapid
236
socioeconomic
237
Valley and the southern bank of the Mediterranean in the first decade of the 21st
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century.
239
•
development (e.g., due to booming oil price) along the Nile
Similar circumstances can be found in East Asia (Figure 3b), where China, South
240
Korea, and Japan represent different stages of socioeconomic development from
241
1992 to 2008. China is still undergoing a rapid development process (the bright
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blue spots), so both the absolute anthropogenic stocks and its spatial distribution
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have greatly increased. While in South Korea, we see large regions in bright white
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or green, which indicates a major increase of anthropogenic stocks from 1992 to
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2000. Japan shows a high and stable anthropogenic stocks distribution across the
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country (all the bright white areas), as it had reached rather high level of
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development at an earlier time before 1992. With the continuing urbanization and
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industrialization, East Asia has reached approximately the same level of
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anthropogenic stocks as Europe (averagely over 40,000 tons/km2).
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•
The Greater Lakes region (Figure 3c) has shown a rather widely and evenly
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distributed pattern of anthropogenic stock, due to its early history of urbanization
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and industrialization. These areas are highly populated and urbanized and have
253
dense transportation networks, resulting in a stock level as high as 59,000
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tons/km2.
255
•
In the Middle East (Figure 3d), where deserts and barren lands could not support
256
many human settlements, the anthropogenic stocks appear much less. Only the oil
257
producing regions near the Persian Gulf and some parts of Saudi Arabia show
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relatively high deposits of anthropogenic stocks. In particular, cities like Dubai
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and Abu Dhabi show a clear pattern of stock increase, owing to their
260
diversification industry strategies (for non-oil economy) and heavy investments on
261
real estate and tourism. On the contrary, a few places (the red spots in Figure 3d)
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in the Middle East and northeast Africa (e.g., in Iraq, Iran, and Sudan) witnessed a
263
decrease of anthropogenic stocks, assumedly due to destruction caused by wars.
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Figure 3. RGB (red, green, blue) composite images for the
2008
spatial-temporal dynamics of regional anthropogenic stocks. 2000
The red band is for the year 1992, green band is for the year 1992
2000, and the blue band is for the year 2008. a) Southern Europe and North Africa; b) East Asia; c) Part of the USA and Canada; d) Middle East near the Persian Gulf.
264 265
3.2 Drivers behind the growth of anthropogenic stocks. The regional differences of
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anthropogenic stocks at more geographically refined levels than earlier global and
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national estimates shown in Figures 2 and 3 may reflect a combined effect of physical
268
geography (e.g., terrain conditions, local climate, and resource availability),
269
architectural and construction specifications (e.g., materials choice and architectural
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style), and socioeconomic development (e.g., economy and stages and models of
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urbanization), though a quantitative analysis of these drivers is not possible.
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Figure 4 shows the distribution of anthropogenic stocks of a few selected metropolitan
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areas at a higher resolution. Figure 4a and 4b demonstrate clear results of
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transit-oriented development: anthropogenic stocks congregate along the rail networks
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(including Shinkansen) in the Kanto region of Japan and along the coastal ports (e.g.,
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Ancona, Ravenna, and Venice) and their connecting railway lines in Northeastern Italy.
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The Tokyo (Figure 4a) and New York metropolitan areas (Figure 4c) contain multiple
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closely-connected urban agglomerations with high anthropogenic stocks, reflecting
280
the dense buildings (e.g., steel skyscrapers) and infrastructure (e.g., over 750
281
passenger cars per 1000 people in the US), high and even socioeconomic
282
development, and terrain conditions (vast plains) in these urbanized areas. On the
283
contrary, Figure 4d shows that anthropogenic stocks distribute more in the city centers
284
in Beijing and Tianjin than sub-urbans and surrounding rural areas, which are still
285
experiencing a rapid expansion process.
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Roads/ routes
railway
10,000
30,000
tons 58, 58,000
Figure 4. High-resolution mapping of anthropogenic stocks in 2008 for selected areas: (a) Kanto region of Japan, around the Greater Tokyo area; (b) Northeastern Italy, along the western coast of the Adriatic Sea; (c) Eastern United States, around the New York Metropolitan area; and (d) the Beijing-Tianjin-Hebei Metropolitan region, China. 287 288
3.3 Robustness and uncertainty of our estimation. Our results provide a first crude
289
estimate of the global anthropogenic stocks on a high resolution level (1 by 1 km) and
290
a fast-estimation technique based on night-time light images with much less data and
291
time cost. These results, of course, bear unavoidably uncertainties from both
292
nighttime light data handling and its correlation with anthropogenic stocks.
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First, the full nighttime light saturation effect27 in city centers could not be fully
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solved without additional urban related data, and we had to adopt a natural city
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extraction concept to limit our stock analysis in the urban areas.
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Second, nighttime lights reflect only patterns of anthropogenic stocks above
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ground but can hardly indicate the amount of anthropogenic stocks underground
298
(such as tunnels and pipelines).
299
Third, the robustness of the power function correlations between anthropogenic
300
stocks and nighttime lights vary by material (e.g., less robust for cement than
301
iron), by sub-category of stocks (e.g., less robust for mobile stocks such as
302
consumer goods than buildings and infrastructure), and by region at different
303
economic development levels (we normalized the nighttime light and stock
304
values by total natural city area to reduce regional difference); therefore such a
305
correction established on the country scale may be imprecise in reflecting both
306
heterogeneity of countries and global unitarity.
307
Lastly but most importantly, scale effect occurs when downscaling the regression
308
relationship established at the country/regional level to grid levels. Although our
309
results reach a best resolution of 1 by 1 km in the present circumstances,
310
comprehensive validation is not possible due to lack of primary data at higher
311
resolution (values are heterogeneous even under 1km grid level).
312 313
In short, these generated data should be interpreted with care at a high-resolution level.
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More empirical case studies on anthropogenic stocks at sub-country, city, or sub-city
315
levels and improved data and methods on nighttime light handling could help address
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these limitations and improve gridded anthropogenic data in the future.
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Nevertheless, the overall spatial-temporal trends and fine-resolution values are
319
reasonable. For example, on the country level, our estimated results of anthropogenic
320
aluminium stock of China in 2005 agree to that mentioned by Gerst and Graedel39
321
within a range of 10%, and our results of anthropogenic cement stock of the U.S. in
322
2000 is consistent with Kapur et al.40 within 5%. Moreover, our results are in good
323
accordance (differing from 9% to 32% in Table 1) with the few earlier studies at a
324
sub-country level (e.g., from district to city to province). These differences are
325
encouraging considering the level of details we provided.
326
Table 1. Comparison between our results with previous estimates Region/City
Year
Material
Connecticut, US
2000
Aluminium
Salford Quays, Manchester, UK Wakayama city centre, Japan Hannan, China Chinese provinces
2000
Cement
327
200841); bottom-up (Tanikawa and 42
Hashimoto 2009 )
This study
Difference
0.9 Mt
25%
~ 35, 000 tons/km2
13%
~0.86 Mt a (Tanikawa 2004
Cement
and Hashimoto
0.75 Mt
13%
0.155 Mt
9%
42
2009 ) 2005
Aluminium
2008
Steel
2010
and civil engineering only)
Vienna, Austria
1.2 Mt (Recalde et al. ~40, 000 tons/km2
Steel (buildings Aichi, Japan
Earlier estimate
2013
0.17 Mt (Lou and Shi 200843); bottom-up ~ 300 Mt on average 26
(Liang et al. 2014 ) ~39 Mt (Liang et al. 201644)
~270 Mt on average ~33 Mt (total stock;
5.9 Mt (Kleemann et.
4 Mt (total
only)
al 201645); bottom-up
stock; 2008)
328
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15%
2008)
Steel (buildings
Note: a. Based on a concrete-to-cement conversion factor of 8.4.
10%
32%
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329
3.4 Implications and discussion. More spatially refined anthropogenic stocks
330
information we generated has significant implications for facilitating more in-depth
331
research on resource management and urban sustainability and supporting policy
332
discussion on resource and environmental sustainability, especially at regional and
333
urban scales.
334
•
Resource recovery via urban mining becomes increasingly important in the
335
circular economy and climate policy agenda worldwide. However, our
336
understanding of the quantity, quality, age, and location of urban mines is still
337
much poorer comparing to that of underground mines. Such a spatially refined
338
mapping of anthropogenic stocks could provide quantitative guidance on
339
potentials (e.g., quality and location) and costs (e.g., transportation costs) for
340
construction industry, demolition companies, and waste handlers. Since
341
anthropogenic stock covers the total amount of material quantities that have been
342
identified through prospection and exploration (often using models), regardless
343
their economic feasibility to retrieve under certain conditions, further research on
344
the “reserves” of urban mines (vis-à-vis geological reserves) is urgently needed.
345
•
Urbanization induced building and infrastructure development couples human
346
well-being development (e.g., shelter and mobility) and environmental impacts
347
along their entire life cycle from construction, maintenance, use, to end-of-life
348
management. Characterization of the these anthropogenic stocks on a high
349
geographical resolution could connect the previously disconnected research fields
350
on their direct impacts in use (e.g., urban geography on transportation behavior
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and work-live spaces) and indirect impacts embodied in materials production and
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construction (e.g., industrial ecology on life cycle environmental impacts). This
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could potentially open up a new line of research that enables transformative,
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dynamic, and integrative understanding of urban sustainability and provide a full
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exploration of dematerialization and decarbonization strategies for cities.
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•
Stock growth patterns vary in different countries and cities. Previous
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understanding on the socioeconomic drivers behind these stock patterns exists
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only on the global and national levels. The anthropogenic stocks data on a more
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refined level could help explore patterns and drivers (e.g., urban form and
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transportation mode) of stock growth from a micro view and thus provide
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benchmark for development of less developed regions and cities.
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•
Cities are the core of both problems and solutions to global sustainability
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challenges. Traditional urban sustainability indicators are based exclusively on
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flow parameters such as water, energy, emissions, and income. Growing
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information on anthropogenic stocks at the city or sub-city level could facilitate
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the establishment of urban sustainability indicators from a critical, but hitherto
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largely overlooked, stock perspective (e.g., the weight of cities), which could
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complement the current array of urban sustainability indicators and related policy.
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AUTHOR INFORMATION
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Corresponding Author
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Environmental Science & Technology
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*Phone: + 45 65509441; e-mail:
[email protected],
[email protected], and
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[email protected].
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ORCID
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Gang Liu: 0000-0002-7613-1985
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Notes
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The authors declare no competing financial interest.
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ASSOCIATED CONTENT
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Supporting Information. Supplementary data and figures on the regression and
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gridded anthropogenic stock results by material by year, and link to freely available
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GeoTIFF format files for all the anthropogenic stocks estimation results in Havard
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Dataverse46. The Supporting Information is available free of charge on the ACS
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Publications website at DOI: XXX.
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ACKNOWLEDGEMENTS
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We acknowledge financial support from National Natural Science Foundation of
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China (41728002, 41471449, 41871331, and 41801343), Independent Research Fund
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Denmark (CityWeight, 6111-00555B), and the Innovation Program of Shanghai
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Municipal Education Commission (15ZZ026).
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